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Beilstein J. Org. Chem. 2017, 13, 2374–2384, doi:10.3762/bjoc.13.235
Graphical Abstract
Figure 1: General structure of investigated DPP derivatives 1–5.
Scheme 1: Synthesis of target DPP chromophores 1–5. (i) PdCl2(PPh3)2, Na2CO3, THF, H2O; (ii) PdCl2(PPh3)2, TH...
Figure 2: Thermograms of representative chromophores 4a and 4b.
Figure 3: Energy level diagram of the electrochemical (black) and DFT (red) derived energies of the EHOMO/LUMO...
Figure 4: UV–vis absorption spectra of chromophores 1a and 1b in 1,4-dioxane at a concentration of 1 × 10−5 M....
Figure 5: UV–vis absorption spectra of chromophores 1b–5b in 1,4-dioxane at a concentration of 1 × 10−5 M.
Figure 6: Typical THG dependences vs the fundamental energy density.
Figure 7: HOMO (red) and LUMO (blue) localizations in 1a (ethylhexyl chains truncated).